Please use this identifier to cite or link to this item: http://hdl.handle.net/1843/44018
Type: Artigo de Periódico
Title: Anomalous non-linear optical response of graphene near phonon resonances
Authors: Lucas Lafetá Prates da Fonseca
Alisson Ronieri Cadore
Thiago Grasiano Mendes de Sá
Kenji Watanabe
Takashi Taniguchi
Leonardo Cristiano Campos
Ado Jorio de Vasconcelos
Leandro Malard Moreira
Abstract: In this work we probe the third-order nonlinear optical property of graphene and hexagonal boron nitride and their heterostructure by the use of coherent anti-Stokes Raman spectroscopy. When the energy difference of the two input fields matches the phonon energy, the anti-Stokes emission intensity is enhanced in h-BN, as usually expected, while for graphene an anomalous decrease is observed. This behavior can be understood in terms of a coupling between the electronic continuum and a discrete phonon state. We have also measured a graphene/h-BN heterostructure and demonstrate that the anomalous effect in graphene dominates the heterostructure nonlinear optical response.
Subject: Ótica não-linear
Grafeno
language: eng
metadata.dc.publisher.country: Brasil
Publisher: Universidade Federal de Minas Gerais
Publisher Initials: UFMG
metadata.dc.publisher.department: ICX - DEPARTAMENTO DE FÍSICA
Rights: Acesso Restrito
metadata.dc.identifier.doi: https://doi.org/10.1021/acs.nanolett.7b00329
URI: http://hdl.handle.net/1843/44018
Issue Date: 25-May-2017
metadata.dc.url.externa: https://pubs.acs.org/doi/10.1021/acs.nanolett.7b00329
metadata.dc.relation.ispartof: Nano Letters
Appears in Collections:Artigo de Periódico

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