Please use this identifier to cite or link to this item: http://hdl.handle.net/1843/64200
Type: Artigo de Periódico
Title: Graphene electromechanical water sensor: the wetristor
Authors: Leonel Muniz Meireles
Bernardo Ruegger Almeida Neves
Leonardo Cristiano Campos
Rodrigo Gribel Lacerda
Eliel Gomes da Silva Neto
Gustavo Arrighi Ferrari
Paulo A. A. Neves
Andreij de Carvalho Gadelha
Ive Silvestre de Almeida
Takashi Taniguchi
Kenji Watanabe
Helio Chacham
Abstract: A water-induced electromechanical response in suspended graphene atop a microfluidic channel is reported. The graphene membrane resistivity rapidly decreases to ≈25% upon water injection into the channel, defining a sensitive “channel wetting” device—a wetristor. The physical mechanism of the wetristor operation is investigated using two graphene membrane geometries, either uncovered or covered by an inert and rigid lid (hexagonal boron nitride multilayer or poly(methyl methacrylate) film). The wetristor effect, namely the water-induced resistivity collapse, occurs in uncovered devices only. Atomic force microscopy and Raman spectroscopy indicate substantial morphology changes of graphene membranes in such devices, while covered membranes suffer no changes, upon channel water filling. The results suggest an electromechanical nature for the wetristor effect, where the resistivity reduction is caused by unwrinkling of the graphene membrane through channel filling, with an eventual direct doping caused by water being of much smaller magnitude, if any. The wetristor device should find useful sensing applications in general micro- and nanofluidics.
Subject: Grafeno
language: eng
metadata.dc.publisher.country: Brasil
Publisher: Universidade Federal de Minas Gerais
Publisher Initials: UFMG
metadata.dc.publisher.department: ICX - DEPARTAMENTO DE FÍSICA
Rights: Acesso Restrito
metadata.dc.identifier.doi: https://doi.org/10.1002/aelm.201901167
URI: http://hdl.handle.net/1843/64200
Issue Date: 2019
metadata.dc.url.externa: https://onlinelibrary.wiley.com/doi/full/10.1002/aelm.201901167
metadata.dc.relation.ispartof: Advanced Functional Materials
Appears in Collections:Artigo de Periódico

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