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Please use this identifier to cite or link to this item: http://hdl.handle.net/1843/68397
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dc.creatorAmanda Aline Barbozapt_BR
dc.creatorJuliana Arantes Dantaspt_BR
dc.creatorGuilherme Augusto de Melo Jardimpt_BR
dc.creatorAttilio Chiavegatti Netopt_BR
dc.creatorWillian Xerxes Coelho Oliveirapt_BR
dc.creatorTobias Genschpt_BR
dc.creatorMarco Antonio Barbosa Ferreirapt_BR
dc.date.accessioned2024-05-16T12:50:57Z-
dc.date.available2024-05-16T12:50:57Z-
dc.date.issued2022-
dc.citation.volume14pt_BR
dc.citation.issue20pt_BR
dc.citation.epagehttps://doi.org/10.1002/cctc.202200894pt_BR
dc.identifier.doihttps://doi.org/10.1002/cctc.202200894pt_BR
dc.identifier.issn1867-3899pt_BR
dc.identifier.urihttp://hdl.handle.net/1843/68397-
dc.description.resumoA Pd-catalyzed heterocyclization/carbonylation cascade reaction encompassing the formation of 3 new bonds, affording dihydropyrazole-esters in moderate to excellent yields and good functional group tolerance is described, comprising a new methodology for direct access to esterified heterocycles using alcohols as readily available feedstock. Optimization was carried out along with a phosphine/base parameterization study, providing important structure-reactivity insights for pyridine-bases, mono- and bisphosphines.pt_BR
dc.description.sponsorshipCNPq - Conselho Nacional de Desenvolvimento Científico e Tecnológicopt_BR
dc.description.sponsorshipCAPES - Coordenação de Aperfeiçoamento de Pessoal de Nível Superiorpt_BR
dc.description.sponsorshipFAPESP - Fundação de Amparo à Pesquisa do Estado de São Paulopt_BR
dc.description.sponsorshipOutra Agênciapt_BR
dc.languageengpt_BR
dc.publisherUniversidade Federal de Minas Geraispt_BR
dc.publisher.countryBrasilpt_BR
dc.publisher.departmentICX - DEPARTAMENTO DE QUÍMICApt_BR
dc.publisher.initialsUFMGpt_BR
dc.relation.ispartofChemCatChempt_BR
dc.rightsAcesso Restritopt_BR
dc.subjectPalladium catalysispt_BR
dc.subjectHeterocyclizationpt_BR
dc.subjectCarbonylationpt_BR
dc.subjectParameterization studiespt_BR
dc.subjectCascade cyclizationpt_BR
dc.subject.otherCatálisept_BR
dc.subject.otherReações quimicaspt_BR
dc.subject.otherFormação de aneis (Quimica)pt_BR
dc.subject.otherCompostos heterociclicospt_BR
dc.subject.otherFosfinapt_BR
dc.subject.otherPiridinapt_BR
dc.titleSynthesis of dihydropyrazoles via Pd-catalyzed heterocyclization/carbonylation reaction: development and parameterization studiespt_BR
dc.typeArtigo de Periódicopt_BR
dc.url.externahttps://chemistry-europe.onlinelibrary.wiley.com/doi/10.1002/cctc.202200894pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0001-5606-911Xpt_BR
dc.identifier.orcidhttps://orcid.org/0000-0003-2473-4167pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-9882-3085pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-4266-4409pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0003-0722-5352pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-1937-0285pt_BR
dc.identifier.orcidhttps://orcid.org/0000-0002-4954-6691pt_BR
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