Interplay of crystalline strain and electronic properties in topological insulators and semiconductor thin films grown by Molecular Beam Epitaxy

dc.creatorGilberto Rodrigues da Silva Junior
dc.date.accessioned2023-05-22T12:08:17Z
dc.date.accessioned2025-09-09T01:04:58Z
dc.date.available2023-05-22T12:08:17Z
dc.date.issued2022-04-29
dc.description.sponsorshipCNPq - Conselho Nacional de Desenvolvimento Científico e Tecnológico
dc.description.sponsorshipCAPES - Coordenação de Aperfeiçoamento de Pessoal de Nível Superior
dc.identifier.urihttps://hdl.handle.net/1843/53715
dc.languageeng
dc.publisherUniversidade Federal de Minas Gerais
dc.rightsAcesso Aberto
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/3.0/pt/
dc.subjectRaios X, difração
dc.subjectEpitaxia por feixe molecular
dc.subjectSemicondutores
dc.subject.otherSynchrotron x-ray diffraction
dc.subject.otherAtomic force microscopy
dc.subject.otherScanning tunneling microscopy/spectroscopy
dc.subject.otherGe condensation
dc.subject.otherBismuth telluride
dc.subject.otherTopological insulators
dc.titleInterplay of crystalline strain and electronic properties in topological insulators and semiconductor thin films grown by Molecular Beam Epitaxy
dc.title.alternativeRelação entre o strain cristalino e propriedades eletrônicas em filmes finos de isolantes topológicos e semicondutores crescidos por Epitaxia de Feixes Moleculares
dc.typeTese de doutorado
local.contributor.advisor1Ângelo Malachias de Souza
local.contributor.advisor1Latteshttp://lattes.cnpq.br/8428074335454256
local.contributor.referee1Myriano Henriques de Oliveira Junior
local.contributor.referee1Ricardo Wagner Nunes
local.contributor.referee1Beatriz Diaz Moreno
local.contributor.referee1Matheus Josué de Souza Matos
local.creator.Latteshttp://lattes.cnpq.br/4121324417549540
local.description.resumoIn this thesis, we studied three different types of samples, all obtained by the molecular beam epitaxy technique (MBE). In the first set of samples, epitaxial layers of Silicon-Germanium (SiGe) after the Germanium condensation process were studied. Our results show that, starting from a low concentration Si0.92Ge0.08 layer grown on top of a crystalline Si (001) on SOI substrates, we can reach desirable Ge concentration with a non-monotonic interplay on in-plane and out-of-plane strain. The Ge concentration and SiGe layer thickness was evaluated by a combination of secondary ion mass spectroscopy (SIMS) and synchotron X-ray measurements (diffraction and reflectivity). In the second set of samples, we have studied the first stages of the heteroepitaxial growth of layered bismuth telluride (Bi2Te3) topological insulator on top of highly oriented pyrolitic graphite (HOPG). Samples were investigated by atomic force microscopy (AFM), synchrotron x-ray diffraction (XRD), and micro-Raman spectroscopy. AFM images show hexagonal/triangular flat islands with exposed HOPG areas for the low coverage regime. The existence of pseudomorphic strain at the initial Bi2Te3 layers was retrieved by both XRD and Raman spectroscopy. Finally, in the third set of samples, we studied the morphological and electronic properties of Bi2Te3 layers doped with Europium (Eu) atoms. Bi2Te3 layers were deposited on a Barium fluoride (BaF2) substrate and characterized by atomic force microscopy (AFM) and scanning tunneling microscopy/spectroscopy (STM/STS) techniques. Our results indicate regions along the sample surface in which the signature of the topological surface states disappears as well as the existence of a second crystalline phase.
local.publisher.countryBrasil
local.publisher.departmentICX - DEPARTAMENTO DE FÍSICA
local.publisher.initialsUFMG
local.publisher.programPrograma de Pós-Graduação em Física

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