Enhanced electronic transport properties of Te roll-like nanostructures

dc.creatorEmilson Ribeiro Viana Junior
dc.creatorNestor Cifuentes Taborda
dc.creatorJuan Carlos González Pérez
dc.date.accessioned2025-02-25T15:07:27Z
dc.date.accessioned2025-09-08T23:40:12Z
dc.date.available2025-02-25T15:07:27Z
dc.date.issued2022
dc.description.sponsorshipCNPq - Conselho Nacional de Desenvolvimento Científico e Tecnológico
dc.description.sponsorshipFAPEMIG - Fundação de Amparo à Pesquisa do Estado de Minas Gerais
dc.description.sponsorshipCAPES - Coordenação de Aperfeiçoamento de Pessoal de Nível Superior
dc.format.mimetypepdf
dc.identifier.doihttps://doi.org/10.3762/bjnano.13.106
dc.identifier.issn2190-4286
dc.identifier.urihttps://hdl.handle.net/1843/80414
dc.languageeng
dc.publisherUniversidade Federal de Minas Gerais
dc.relation.ispartofBeilstein Journal of Nanotechnology
dc.rightsAcesso Aberto
dc.subjectTellurium
dc.subjectNanoestrutura
dc.subjectMicroscopia eletrônica de varredura
dc.subject.otherElectrical characterization
dc.subject.otherField-effect transistors
dc.subject.otherHopping conduction
dc.subject.otherNanobelts
dc.subject.otherTellurium
dc.titleEnhanced electronic transport properties of Te roll-like nanostructures
dc.typeArtigo de periódico
local.citation.epage1291
local.citation.spage1284
local.citation.volume13
local.description.resumoIn this work, the electronic transport properties of Te roll-like nanostructures were investigated in a broad temperature range by fabricating single-nanostructure back-gated field-effect-transistors via photolithography. These one-dimensional nanostructures, with a unique roll-like morphology, were produced by a facile synthesis and extensively studied by scanning and transmission electron microscopy. The nanostructures are made of pure and crystalline Tellurium with trigonal structure (t-Te), and exhibit p-type conductivity with enhanced field-effect hole mobility between 273 cm2/Vs at 320 K and 881 cm2/Vs at 5 K. The thermal ionization of shallow acceptors, with small ionization energy between 2 and 4 meV, leads to free-hole conduction at high temperatures. The free-hole mobility follows a negative power-law temperature behavior, with an exponent between −1.28 and −1.42, indicating strong phonon scattering in this temperature range. At lower temperatures, the electronic conduction is dominated by nearest-neighbor hopping (NNH) conduction in the acceptor band, with a small activation energy ENNH ≈ 0.6 meV and an acceptor concentration of NA ≈ 1 × 1016 cm−3. These results demonstrate the enhanced electrical properties of these nanostructures, with a small disorder, and superior quality for nanodevice applications.
local.identifier.orcidhttps://orcid.org/0000-0002-1883-3508
local.identifier.orcidhttps://orcid.org/0000-0003-3638-7959
local.identifier.orcidhttps://orcid.org/0000-0001-9155-1657
local.publisher.countryBrasil
local.publisher.departmentICX - DEPARTAMENTO DE FÍSICA
local.publisher.initialsUFMG
local.url.externahttps://www.beilstein-journals.org/bjnano/articles/13/106

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