Electromechanical modulations in transition metal dichalcogenide nanosheets: implications for environmental sensors

dc.creatorMauricio Vasconcelos Bessa
dc.creatorWellington Damaceno de Freitas
dc.creatorNatália Paz Neme
dc.creatorLuiz Gustavo Pimenta Martins
dc.creatorAna Paula Moreira Barboza
dc.creatorMatheus Josué de Souza Matos
dc.creatorMario Sergio de Carvalho Mazzoni
dc.creatorBernardo Ruegger Almeida Neves
dc.date.accessioned2025-07-16T18:34:20Z
dc.date.accessioned2025-09-09T00:40:28Z
dc.date.available2025-07-16T18:34:20Z
dc.date.issued2021
dc.description.sponsorshipCNPq - Conselho Nacional de Desenvolvimento Científico e Tecnológico
dc.description.sponsorshipFAPEMIG - Fundação de Amparo à Pesquisa do Estado de Minas Gerais
dc.description.sponsorshipINCT – Instituto nacional de ciência e tecnologia (Antigo Instituto do Milênio)
dc.identifier.doihttps://doi.org/10.1021/acsanm.1c03002
dc.identifier.issn2574-0970
dc.identifier.urihttps://hdl.handle.net/1843/83584
dc.languageeng
dc.publisherUniversidade Federal de Minas Gerais
dc.relation.ispartofACS Applied Nano Materials
dc.rightsAcesso Restrito
dc.subjectScanning probe microscopy
dc.subjectTeoria do Funcional da Densidade
dc.subjectPressão
dc.subject.other2D materials
dc.subject.otherPressure-induced structural transition
dc.subject.otherTransition metal dichalcogenides
dc.subject.otherScanning probe microscopy
dc.subject.otherPressure
dc.titleElectromechanical modulations in transition metal dichalcogenide nanosheets: implications for environmental sensors
dc.typeArtigo de periódico
local.citation.epage11311
local.citation.issue10
local.citation.spage11305
local.citation.volume4
local.description.resumoTransition metal dichalcogenides (TMDs) are key players in the two-dimensional materials nanoarena due to their exquisite optoelectronic properties under a standard environment (room temperature and atmospheric pressure). Nevertheless, as reported in the literature, they may also portray interesting physical properties under different environments. Here, we show two distinct and significant electromechanical modulations in TMD nanosheets which are tuned by the environmental conditions (applied pressure and adsorbents). Using scanning probe microscopy techniques, we modify the environmental conditions and observe steplike rises in the electrical response of all studied TMDs (MoS 2 , WS 2, MoSe2, and WSe 2 - monolayers and few layers). Ab initio calculations enable full understanding of specific mechanisms behind these electromechanical modulations, which may find important applications in the design of TMD-based environmental sensors.
local.identifier.orcidhttps://orcid.org/0000-0002-7978-2134
local.identifier.orcidhttps://orcid.org/0000-0001-9777-7999
local.identifier.orcidhttps://orcid.org/0000-0002-1807-971X
local.identifier.orcidhttps://orcid.org/0000-0002-0398-3992
local.identifier.orcidhttps://orcid.org/0000-0001-5897-6936
local.identifier.orcidhttps://orcid.org/0000-0003-0464-4754
local.publisher.countryBrasil
local.publisher.departmentICX - DEPARTAMENTO DE FÍSICA
local.publisher.initialsUFMG
local.url.externahttps://pubs.acs.org/doi/10.1021/acsanm.1c03002

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